Plasmon-assisted photoelectron emission in a model cluster using time-dependent density functional theory and the time-dependent surface-flux method
Published: Jul 30, 2025
Last Updated: Jul 30, 2025
Authors:Mikhail Bednov, Waqas Pervez, Ingo Barke, Dieter Bauer
Abstract
We investigate plasmon-assisted photoelectron emission using a one-dimensional time-dependent density-functional theory (TDDFT) model. Photoelectron spectra are computed with the time-dependent surface-flux (t-SURFF) method. In addition to the expected above-threshold ionization (ATI) comb, we observe peaks that arise from long-lived plasmon oscillations and the associated electron emission occurring after the laser pulse. We further analyze the positions of these peaks and their scaling behavior with the laser intensity.