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Boron-doped diamond crystals (BDD, C$_{1-x}$B$_{x}$) exhibit exceptional mechanical strength, electronic tunability, and resistance to radiation damage. This makes them promising materials for use in gamma-ray crystal-based light sources. To better understand and quantify the structural distortions introduced by doping, which are critical for maintaining channelling efficiency, we perform atomistic-level molecular dynamics simulations on periodic C$_{1-x}$B$_{x}$ systems of various sizes. These simulations allow the influence of boron concentration on the lattice constant and the (110) and (100) inter-planar distances to be evaluated over the concentration range from pure diamond (0%) to 5% boron at room temperature (300 K). Linear relationships between both lattice constant and inter-planar distance with increasing dopant concentration are observed, with a deviation from Vegard's Law. This deviation is larger than that reported by other theoretical and computational studies; however, this may be attributed to an enhanced crystal quality over these studies, a vital aspect when considering gamma-ray crystal light source design. The methodology presented here incorporates several refinements to closely reflect the conditions of microwave plasma chemical vapour deposition (MPCVD) crystal growth. Validation of the methodology is provided through a comprehensive statistical analysis of the structure of our generated crystals. These results enable reliable atomistic modelling of doped diamond crystals and support their use in the design and fabrication of periodically bent structures for next-generation gamma-ray light source technologies.
We present a method for determining the azimuthal phase (angle) of a magnetic field by exploiting phase matching of laser beams in a ground-state Hanle effect (GHSE) configuration. This approach is based on the symmetry of the system's Hamiltonian and the existence of a phase-independent frame, allowing for direct determination of the field orientation. As a proof of concept, we performed preliminary experiments using the Fg=1 to Fe=0 transition of the D2 line in 87Rb, with three laser beams to demonstrate the phase (azimuthal) dependence of the observed Hanle resonance signals. While our current setup does not include active phase control, the key features predicted by our method were observed, validating its conceptual foundation. Additionally, we measured two components of the stray magnetic field in our laboratory as an illustration. This method leverages the Hanle effect's inherent sensitivity to both the magnitude and orientation of magnetic fields, as well as the underlying symmetry properties of the atomic system, and offers a pathway for precise, calibration-free determination of magnetic field orientation.
High-harmonic spectroscopy (HHS) in liquids promises real-time access to ultrafast electronic dynamics in the native environment of chemical and biological processes. While electron recollision has been established as the dominant mechanism of high-harmonic generation (HHG) in liquids, resolving the underlying electron dynamics has remained elusive. Here we demonstrate attosecond-resolved measurements of recolliding electron wave packets, extending HHS from neat liquids to aqueous solutions. Using phase-controlled two-colour fields, we observe a linear scaling of the two-colour delay that maximizes even-harmonic emission with photon energy, yielding slopes of 208+/-55 as/eV in ethanol and 124+/-42 as/eV in water, the latter matching ab initio simulations (125+/-48 as/eV). In aqueous salt solutions, we uncover interference minima whose appearance depends on solute type and concentration, arising from destructive interference between solute and solvent emission. By measuring the relative phase of solvent and solute HHG, we retrieve a variation of electron transit time by 113+/-32 as/eV, consistent with our neat-liquid results. These findings establish HHS as a powerful attosecond-resolved probe of electron dynamics in disordered media, opening transformative opportunities for studying ultrafast processes such as energy transfer, charge migration, and proton dynamics in liquids and solutions.
We investigate the dynamical phase evolution of Coulomb-focused electrons in strong-field ionization. We diffract the electrons with an ultrashort standing light wave to track their time-dependent phase. Our findings show that low-energy electrons exhibit a unique chromosome-shaped diffraction pattern, distinct from higher-energy electrons. Our numerical model quantitatively reproduces the experimental results, confirming this pattern maps the electron's time-dependent phase evolution as it escapes from a Coulomb potential. Our pulsed diffraction grating technique offers a new way to sense an electron's quantum phase without interfering its release mechanism.
We present a MATLAB script which can use GPU acceleration to simulate a trapped ion interacting with a low-density cloud of atoms. This script, called atomiongpu.m, can massively parallelize MD simulations of trajectories of a trapped ion and an atom starting far away. The script uses ode45gpu, which is our optimized and specialized implementation of the Runge-Kutta algorithm used in MATLAB's ODE solver ode45. We first discuss the physical system and show how ode45gpu can solve it up to 22x faster than MATLAB's ode45. Then, we show how to easily modify the inputs to atomiongpu.m to account for different kinds of atoms, ions, atom-ion interactions, trap potentials, simulation parameters, initial conditions, and computational hardware, so that atomiongpu.m automatically finds the probability of complex formation, the distribution of observables such as the scattering angle and complex lifetime, and plots of specific trajectories.
Landau levels (LLs) are the massively-degenerate discrete energy spectrum of a charged particle in a transverse magnetic field and lie at the heart of many intriguing phenomena such as the integer and fractional quantum Hall effects as well as quantized vortices. In this Letter, we consider coupling of LLs of a transversely driven charge neutral particle in a synthetic gauge potential to a quantized field of an optical cavity -- a setting reminiscent of superradiant self-ordering setups in quantum gases. We uncover that this complex system can be surprisingly described in terms of two highly nonlinearly-coupled quantum harmonic oscillators, thus enabling a full quantum mechanical treatment. Light-matter coupling mixes the LLs and the superradiant photonic mode, leading to the formation of hybrid states referred to as ``Landau polaritons''. They inherit partially the degeneracy of the LLs and possess intriguing features such as non-zero light-matter entanglement and quadrature squeezing. Depending on the system parameters and the choice of initial state, the system exhibits diverse nonequilibrium quantum dynamics and multiple steady states, with distinct physical properties. This work lays the foundation for further investigating the novel, driven-dissipative Landau-polariton physics in quantum-gas--cavity-QED settings.
The Hopfield model describes a neural network that stores memories using all-to-all-coupled spins. Memory patterns are recalled under equilibrium dynamics. Storing too many patterns breaks the associative recall process because frustration causes an exponential number of spurious patterns to arise as the network becomes a spin glass. Despite this, memory recall in a spin glass can be restored, and even enhanced, under quantum-optical nonequilibrium dynamics because spurious patterns can now serve as reliable memories. We experimentally observe associative memory with high storage capacity in a driven-dissipative spin glass made of atoms and photons. The capacity surpasses the Hopfield limit by up to seven-fold in a sixteen-spin network. Atomic motion boosts capacity by dynamically modifying connectivity akin to short-term synaptic plasticity in neural networks, realizing a precursor to learning in a quantum-optical system.
We present a geometric interpretation of the hyperfine Breit--Rabi eigenvalues and eigenvectors in alkali atoms after reformulating the standard solution into a compact form. In this picture, the nuclear magnetic moment has a polar angle fixed by the total projection quantum number. In contrast, the electron magnetic moment anti-aligns or aligns with an effective field formed by both the external magnetic flux density and the nuclear field, which simultaneously sets the mixing angle of the eigenvectors. This geometric view offers intuitive insight into the structure of the solutions.
Arrays of neutral atoms present a promising system for quantum computing, quantum sensors, and other applications, several of which would profit from the ability to load, cool, and image the atoms in a finite magnetic field. In this work, we develop a technique to image and prepare $^{87}$Rb atom arrays in a finite magnetic field by combining EIT cooling with fluorescence imaging. We achieve 99.6(3)% readout fidelity at 98.2(3)% survival probability and up to 68(2)% single-atom stochastic loading probability. We further develop a model to predict the survival probability, which also agrees well with several other atom array experiments. Our technique cools both the axial and radial directions, and will enable future continuously-operated neutral atom quantum processors and quantum sensors.
Cold atoms are promising platforms for metrology and quantum computation, yet their many-body dynamics remains largely unexplored. We here investigate Rabi oscillations from optically-thick cold clouds, driven by high-intensity coherent light. A dynamical displacement from the atomic resonance is predicted, which can be detected through the collective Rabi oscillations of the atomic ensemble. Different from linear-optics shifts, this dynamical displacement grows quadratically with the optical depth, yet it reduces with increasing pump power as dipole-dipole interactions are less effective. This modification may be particularly important for Ramsey spectroscopy, when strong pulses and optically dense samples are used.
We propose an O(100)m Atom Interferometer (AI) experiment - AICE - to be installed against a wall of the PX46 access shaft to the LHC. This experiment would probe unexplored ranges of the possible couplings of bosonic ultralight dark matter (ULDM) to atomic constituents and undertake a pioneering search for gravitational waves (GWs) at frequencies intermediate between those to which existing and planned experiments are sensitive, among other fundamental physics studies. A conceptual feasibility study showed that this AI experiment could be isolated from the LHC by installing a shielding wall in the TX46 gallery, and surveyed issues related to the proximity of the LHC machine, finding no technical obstacles. A detailed technical implementation study has shown that the preparatory civil-engineering work, installation of bespoke radiation shielding, deployment of access-control systems and safety alarms, and installation of an elevator platform could be carried out during LS3, allowing installation and operation of the AICE detector to proceed during Run 4 without impacting HL-LHC operation. These studies have established that PX46 is a uniquely promising location for an AI experiment. We foresee that, if the CERN management encourages this Letter of Intent, a significant fraction of the Terrestrial Very Long Baseline Atom Interferometer (TVLBAI) Proto-Collaboration may wish to contribute to AICE.
Rydberg atoms, due to their large polarizabilities and strong transition dipole moments, have been utilized as sensitive electric field sensors. While their capability to detect modulated signals has been previously demonstrated, these studies have largely been limited to laboratory-generated signals tailored specifically for atomic detection. Here, we extend the practical applicability of Rydberg sensors by demonstrating the reception of real-world frequency-modulated (FM) audio transmissions using a consumer-grade handheld two-way radio operating in the UHF band. Detection is based on the AC Stark shift induced by the radio signal in a Rydberg atomic vapor, with demodulation performed using an offset local oscillator and lock-in amplification. We successfully demodulate speech signals and evaluate the audio spectral response and reception range. We show that all consumer-accessible radio channels can be simultaneously detected, and demonstrate simultaneous reception of two neighboring channels with at least 53 dB of isolation. This work underscores the potential of Rydberg atom-based receivers for practical, real-world FM signal detection.
Ji etal [New J. Phys. 26, 093014 (2024)] established a direct link between the photoionization cross section and the attosecond time delay near Cooper minima (CM) in the valence shells of noble-gas atoms. This link is based on the analytic properties of the ionization amplitude in the complex plane of the photoelectron energy, and is particularly sensitive to the winding number of the amplitude around the origin of the complex energy plane. Here, we demonstrate an analogous relation for photoionization of the valence $ns$ shells of alkali-metal atoms (AMA), from Na ($n=3$) to Cs ($n=6$), as well as alkaline-earth-metal atoms (AEMA), from Mg ($n=3$) to Ba ($n=6$). To this end, we employ a fully relativistic formalism that separates the two complementary $ns_{1/2} \to Ep_{1/2}$ and $Ep_{3/2}$ ionization channels. Each of these channels exhibits a phase variation close to $\pi$, but in opposite directions, near their respective Cooper minima. This phase variation vanishes in a nonrelativistic formulation, where the two channels become degenerate. For AMA, due to the threshold proximity of the CM, the universal Coulomb contribution to the time delay must be subtracted. The remaining component of the time delay is target-specific, angular-dependent, and accessible through comparative measurements.
A semi-empirical model is presented for the thermalized temperature $T$ and mean momentum in the direction of laser propagation <$p_{fz}$> of electrons released from O$_{2}$ after the passage of a focused $800$ nm ultrashort pulsed laser pulse vs. peak laser intensity $I_{0}$ to provide initial conditions for electrodynamic fluid simulations. For this, theoretical kinetic energy spectra in different directions are modified with two adjustable parameters representing the effects of electron rescatter off its parent ion during the optical cycle subsequent to ionization. The classical kinematics of rescatter, in conjunction with the spectral fits, is used to estimate <$p_{fz}$>.
In this paper, we present a mathematical analysis of time-dependent $N$-body electronic systems and establish mixed regularity for the corresponding wavefunctions. Based on this, we develop sparse grid approximations to reduce computational complexity, including a sparse grid Gaussian-type orbital (GTO) scheme. We validate the approach on the Helium atom (${\rm He}$) and Hydrogen molecule (${\rm H}_2$), showing that sparse grid GTOs offer an efficient alternative to full grid discretizations.
The FAMU experiment, supported and funded by the Italian Institute of Nuclear Physics (INFN) and by the Science and Technology Facilities Council (STFC), aims to perform the first measurement of the ground-state hyperfine splitting (1S-hfs) of muonic hydrogen ($\mu H$). This quantity is highly sensitive to the proton's Zemach radius $R_Z$. An experimental determination of $R_Z$ provides significant constraints on the parametrization of the proton form factors as well as on theoretical models describing the proton's electromagnetic structure. Following years of technological and methodological development, the FAMU experiment began operations in 2023 at Port 1 of the RIKEN-RAL muon beam line at the ISIS Neutron and Muon Source facility (Didcot, UK). In this paper, we first describe the unique detection technique employed by FAMU to determine the 1S-hfs of muonic hydrogen, followed by a detailed presentation of the final experimental layout. Finally, we report the first outcome from the 2023 commissioning run and from the initial physics runs performed in 2023 and 2024.
The right kind of theoretical treatment of direct Coulomb ionization of inner-shell of target atoms including multiple ionization of their outer-shells by using accurate x-ray fluorescence yield data and electron capture by projectile ions from inner-shell electrons of target atoms enables us to fully understand the complex physics issues with the heavy-ion-induced inner-shell ionization phenomenon. Such great success has only been achieved recently [Phys. Rev. A 111 (2025) 042827]. Aftermath, further investigations exhibit such a picture only if the Fermi velocity of the elemental target is accurate, as it takes a significant role in correct evaluation of charge-state distribution of the projectile ions inside the target, which contributes an invaluable share in calculating the electron capture-induced ionization cross section correctly. In this work, we devise a powerful method that enables us to measure the correct and accurate Fermi velocity for almost every elemental metal in the periodic table. As per our present knowledge, this in turn not only improves our understanding of the said complex physics issues one step ahead but also helps move toward further miniaturization of integrated circuits and use the heavy-ion-induced X-ray emission in impurity analysis more reliable and accurate.
Using both simulation and experiment, we investigate the robustness of dynamical decoupling sequences to pulse errors: rotation errors and detuning errors. Whereas prior work examined the effect of errors on coherence times, here we show that quantum sensing can be affected by pulse errors in dramatically different ways than coherence times alone. We also explore the effects of qubit leakage: off-resonant coupling to other quantum levels. We find order-of-magnitude differences between commonly-used dynamical decoupling sequences in both their sensitivity to pulse errors and leakage.