CyberSec Research

The famous two-fluid model of finite-temperature superfluids has been recently extended to describe the mixed classical-superfluid dynamics of the newly discovered supersolid phase of matter. We show that for rigidly rotating supersolids one can derive a more appropriate single-fluid model, in which the seemingly classical and superfluid contributions to the motion emerge from a spatially varying phase of the global wavefunction. That allows to design experimental protocols to excite and detect the peculiar rotation dynamics of annular supersolids, including partially quantized supercurrents, in which each atom brings less than $\hbar$ unit of angular momentum. Our results are valid for a more general class of density-modulated superfluids.

Time-resolved atom interferometry, as employed in applications such as gravitational wave detection and searches for ultra-light dark matter, requires precise control over systematic effects. In this work, we investigate phase noise arising from shot-to-shot fluctuations in the atoms' transverse motion in the presence of the wavefront curvature of the interferometer beam, and analyse its dependence on the laser-beam geometry in long-baseline, large-momentum-transfer atom interferometers. We use a semi-classical framework to derive analytical expressions for the effective phase perturbation in position-averaged measurements and validate them using Monte Carlo simulations. Applied to 100-m and 1-km atom gradiometers representative of next-generation experiments, the model shows that configurations maximizing pulse efficiency also amplify curvature-induced phase noise, requiring micron-level control of the atom cloud's centre-of-mass position and sub-micron-per-second control of its centre-of-mass velocity to achieve sub-$10^{-5}$ rad phase stability. Alternative beam geometries can suppress this noise by up to two orders of magnitude, but at the cost of reduced pulse efficiency. To address this limitation, we propose a mitigation strategy based on position-resolved phase-shift readout, which empirically learns and corrects the wavefront-induced bias from measurable quantities such as the phase-shift gradient and final cloud position. This approach restores high-sensitivity operation in the maximum-pulse-efficiency configuration without detailed beam characterisation, providing a practical route towards next-generation, time-resolved atom interferometers operating at the $10^{-5}$ rad noise level.

This is a concise, pedagogical introduction to the dynamic field of open quantum systems governed by Markovian master equations. We focus on the mathematical and physical origins of the Lindblad equation, its unraveling in terms of pure-state trajectories, the structure of steady states with emphasis on the role of symmetry and conservation laws, and a sampling of the novel physical phenomena that arise from nonunitary dynamics (dissipation and measurements). This is far from a comprehensive summary of the field. Rather, the objective is to provide a conceptual foundation and physically illuminating examples that are useful to graduate students and researchers entering this subject. There are exercise problems and references for further reading throughout the notes.

Radiation-matter hybridization allows atoms to serve as mediators of effective interactions between light modes and, conversely, to interact among themselves via light. Here we exploit the spatial structure of atomic ensembles to control the coupling between modes of distinct cavities, thereby reshaping the resulting atom-photon spectra. We show that extended homogeneous clouds suppress mode-mode couplings through destructive interference, whereas grated clouds can preserve them under specific Bragg conditions. This leads to mode-mode spectral subsplittings, where collectivity arises not only from the atom number but also from the ability to tune modes of different cavities independently. Our results establish spatially engineered atomic ensembles as a pathway to selective photon transfer between modes and precise control of many-body complexity.

Rydberg atom arrays are a promising platform for quantum optimization, encoding computationally hard problems by reducing them to independent set problems with unit-disk graph topology. In Nguyen et al., PRX Quantum 4, 010316 (2023), a systematic and efficient strategy was introduced to encode multiple problems into a special unit-disk graph: the King's subgraph. However, King's subgraphs are not the optimal choice in two dimensions. Due to the power-law decay of Rydberg interaction strengths, the approximation to unit-disk graphs in real devices is poor, necessitating post-processing that lacks physical interpretability. In this work, we develop an encoding scheme that can universally encode computationally hard problems on triangular lattices, based on our innovative automated gadget search strategy. Numerical simulations demonstrate that quantum optimization on triangular lattices reduces independence-constraint violations by approximately two orders of magnitude compared to King's subgraphs, substantially alleviating the need for post-processing in experiments.

Using an ultracold gas of $^{87}$Rb$^{133}$Cs molecules, we perform hyperfine-resolved spectroscopy of transitions from the vibronic ground state to the lowest rovibrational states of the electronic state $\mathrm{b}^3\Pi_0$, as a function of magnetic field. These transitions are spin forbidden, resulting in narrow linewidths, and feature near-diagonal Franck-Condon factors. We develop a model of the hyperfine and Zeeman structure that includes coupling between the $0^+$ and $0^-$ components of $\mathrm{b}^3\Pi_0$. We fit the spectra to obtain rotational and hyperfine coupling constants. We measure transition dipole moments associated with specific transitions by directly observing Rabi oscillations as a function of a resonant laser pulse duration. Using resonant $\pi$ pulses, we prepare molecules in the electronically excited state and directly measure the spontaneous emission rate.

By critically evaluating higher-order nonlinear effects to the isotope shifts (ISs) in the low-lying transition frequencies of the singly charged calcium ion, stringent constraint on the electron-neutron coupling due to a hypothetical boson describing physics beyond the Standard Model is inferred. It shows an order magnitude difference compared to the previously reported limit demonstrating importance of higher-order effects in the analysis of nonlinearity in the King's plot. The first-order IS parameters and enhancement factor ($D$) were evaluated using two complementary approaches in the relativistic coupled-cluster theory framework: namely finite-field (FF) and analytical response (AR) approaches. Extraction of the second-order IS parameters in the FF approach show numerical instabilities, so they are determined in the AR approach. Comparison of these factors with previous calculation shows substantial differences in the magnitudes. However, $D$ values from both the FF and AR approaches display excellent agreement. We also show explicitly roles of electron correlation effects in the evaluation of $D$ values accurately.

We observe a fast Penning ionization in a dilute gas of cold rubidium Rydberg atoms, in the presence of a static electric field of 50 V/cm, with the ionization rate coefficients for two specific states being measured, which are orders of magnitude higher than the theoretical predictions in field-free space. Our analysis based on a polarized two-atom model reveals that the ionization threshold of Rydberg atoms is lowered by the static electric field, reducing the energy exchange required for Penning ionization and increasing the ionization rate. Beyond this, the dipole-dipole interaction strengthened by the electric field between two Rydberg atoms at a micrometer-scale distance leads to double ionization of the atoms pair, opening a new autoionization channel. Such enhancement of the Penning ionization by a static electric field poses both a threat to the stability and a potential control strategy for quantum systems composed of cold Rydberg atoms with micrometer-scale interatomic separations.

The emergence of order in many-body systems and the associated self-similar dynamics governed by dynamical scaling laws is a hallmark of universality far from equilibrium. Measuring and classifying such nontrivial behavior for novel symmetry classes remains challenging. Here, we realize a well-controlled interlayer coupling quench in a tunable bilayer two-dimensional Bose gas, driving the system to an ordered phase. We observe robust self-similar dynamics and a universal critical exponent consistent with diffusion-like coarsening, driven by vortex and antivortex annihilation induced by the interlayer coupling. Our results extend the understanding of universal dynamics in many-body systems and provide a robust foundation for quantitative tests of nonequilibrium effective field theories.

We investigate the intermolecular interactions between laser-cooled CaF and Ca, in their ground and excited electronic states, aiming to understand atom-exchange reaction pathways. Using state-of-the-art \textit{ab initio} quantum chemistry methods, we compute potential energy surfaces for nine electronic states arising from the lowest three asymptotes of Ca$_2$F trimer, within the rigid rotor approximation applied to CaF. Two-dimensional potential energy surfaces are computed for the ground state and one of the excited states. We use a combination of the coupled cluster method restricted to single, double, and perturbative triple excitations, and the multireference configuration interaction method with single and double excitations. The ground (X)~$^2\mathrm{A}'$ electronic state of the trimer is significantly deep and highly anisotropic. The excited electronic states are also strongly bound. Notably, the potential energy surface of one of the excited states, (2)~$^2\mathrm{A}'$, lies below the ground-state asymptote of the trimer. By analyzing the potential energy surfaces, we discuss atom-exchange reaction pathways involving both the ground-state interaction between CaF and Ca and the excited metastable state of Ca.

This work theoretically investigates possibilities of using the Stimulated Raman Adiabatic Passage (STIRAP) and its variants to control a coherent superposition of quantum states. We present a generalization of the so-called fractional STIRAP (f-STIRAP), demonstrating precise control over the mixing ratio of quantum states in the wave packet. In contrast to conventional f-STIRAP, designed to drive a system from an eigenstate into a coherent superposition, our scheme enables arbitrary control over the composition of an already existing superposition state. We demonstrate that an approximate version of this technique -- where analytically designed laser pulses with composite envelopes are replaced by simple Gaussian pulses -- achieves comparable performance in controlling the dynamics of the wave packet. A limiting case of this scheme, utilizing two pulses with identical Gaussians envelopes and tuned delay and relative phase, is also explored, revealing experimentally accessible pathways for manipulating quantum coherence. We apply our developed techniques to control the ultrafast charge migration in the spin-orbit split ground electronic states of xenon cation via intermediate valence- and core-excited states. Finally, we propose concrete experimental realizations of the developed control schemes in combination with attosecond transient absorption spectroscopy as a method to probe the system.

Non-equilibrium molecular dynamics (NEMD) simulations were used to study pool boiling of water films on an ultra-thin planar aluminum substrate as well as the effect of surface wettability. The simulation geometry is a 10 nm-thick water film on an FCC aluminum substrate heated from 300 K to 900 K. The first peak acceleration onset time of the film, as the measure of the nucleation start, has been observed. The average heating rates of the near-wall water were 0.064, 0.048, and 0.035 K/ps for hydrophilic, neutral, and hydrophobic surfaces, respectively. Boiling curves shows that the critical heat flux (CHF) equals 5216, 3979, and 2525 MW/m^2 at wall temperatures of 466, 502, and 561 K, respectively. The minimum heat flux (MHF, Leidenfrost point) is equal to 2157, 2463, and 2366 MW/m^2 at wall temperatures of 767, 784, and 746 K, respectively. Interfacial HTC remains higher for longer times under the hydrophilic condition, whereas Kapitza resistance is low initially but then increases sharply after transition to film boiling with the highest values for the hydrophobic surface. In general, the results demonstrate that engineering aluminum wettability towards intense hydrophilicity diminishes the explosive boiling point, increases CHF, and enhances nanoscale thermal management performance.

Laser cooling of large, complex molecules is a long-standing goal, instrumental for enabling new quantum technology and precision measurements. A primary consideration for the feasibility of laser cooling, which determines the efficiency and technical requirements of the process, is the number of excited-state decay pathways leading to vibrational excitations. Therefore, the assessment of the laser-cooling potential of a molecule begins with estimate of the vibrational branching ratios of the first few electronic excited states theoretically to find the optimum cooling scheme. Such calculations, typically done within the BO and harmonic approximations, have suggested that one leading candidate for large, polyatomic molecule laser cooling, alkaline earth phenoxides, can most efficiently be laser-cooled via the third electronically excited C state. Here, we report the first detailed spectroscopic characterization of the C state in CaOPh and SrOPh. We find that nonadiabatic couplings between the A, B, and C states lead to substantial mixing, giving rise to vibronic states that enable additional decay pathways. Based on the intensity ratio of these extra decay channels, we estimate a non-adiabatic coupling strength of 0.1 cm-1. While this coupling strength is small, the large density of vibrational states available at photonic energy scales in a polyatomic molecule leads to significant mixing. Thus, this result is expected to be general for large molecules and implies that only the lowest electronic excited state should be considered when judging the suitability of a molecule for laser cooling.

We propose a method for using a single-axis atom interferometric gravity gradiometer to measure off-diagonal elements of the gravity gradient tensor. By tilting the gradiometer, the measured gradient becomes a linear combination of different components of the gravity gradient tensor, and through multiple measurements at different tilts the separate tensor components can be inferred. We present a theoretical and numerical investigation of this technique, both for terrestrial surveys where the tilt is statically set by the user and for surveys where a strapdown sensor is dynamically tilted by the motion of the platform. We show that the gradiometer's sensitivity to the vertical gravity gradient is only slightly reduced by this method while allowing for more gradiometer information to be obtained. Major sources of error and loss of sensitivity on dynamic platforms are shown to be mitigated using an optical-gimbal technique employing commercially-available fibre-optic gyroscopes and tip-tilt mirrors.

We investigate the decay process $5s5p\,{}^1P_1 \to 5s4d\,{}^1D_2 \to 5s5p\,{}^3P_2$ in a magneto-optical trap of Sr atoms operating on the $461\,\mathrm{nm}$ ($5s^2\,{}^1S_0 - 5s5p\,{}^1P_1$) transition by irradiating the trapped atoms with laser light resonant with the $448\,\mathrm{nm}$ ($5s4d\,{}^1D_2 - 5s8p\,{}^1P_1$) transition and observing the transient response of atom fluorescence. We measure, for the first time, the branching ratio of the $5s4d\,{}^1D_2 \to 5s5p\,{}^3P_2$ transition to be $0.177(4)$, which significantly deviates from the widely cited theoretical value of $0.322$ [C. W. Bauschlicher Jr. et al., J. Phys. B 18, 1523 (1985)]. Moreover, we determine the decay rate of the $5s5p\,{}^1P_1 \to 5s4d\,{}^1D_2$ transition to be $5.3(5)\times10^3\,\mathrm{s^{-1}}$, consistent within uncertainty with the widely cited experimental value [L. R. Hunter et al., Phys. Rev. Lett. 56, 823 (1986)], but substantially lower than the recent theoretical value of $9.25(40)\times10^3\,\mathrm{s^{-1}}$ [A. Cooper et al., Phys. Rev. X 8, 041055 (2018)]. These findings have significant implications for laser cooling of Sr and fluorescence detection of single atoms in optical tweezers. They also call for a reevaluation of theoretical frameworks used to calculate transition rates essential for evaluating blackbody radiation shifts in the Sr optical atomic clock.

Here we address the fundamental question whether an idealized system of $N$ atoms will show collective behavior and superradiance when it emits fermions instead of photons. We show that the maximum emission is $\propto N$ and not $\propto N^2$ which proves the absence of superradiance and shows that the recent proposal to realize a superradiant neutrino laser is impossible. This can be understood as either destructive interference of fermionic transition amplitudes, or Pauli blockade by collective excitations with fermionic nature. On the other hand, states with low excitation can show collective behavior. We derive the exact solution of the fermionic Dicke problem and analyze the decay dynamics in various regimes.

This paper lays out the principles of how Bose-Einstein condensates can modify radioactive decay. We highlight the challenges of many modes and short coherence times due to the $\approx$ MeV energies of the emitted radiation. Recent proposals for gamma ray and neutrino lasers claim that using a Bose-Einstein condensate as a source would solve these issues. We show that this is not the case, and the proposed experiments would have a gain of only $10^{-20}$ or smaller. We also analyze proposals for gamma ray lasers based on stimulated annihilation of positronium Bose-Einstein condensates.

Rydberg atomic radio-frequency (rf) sensors are an emerging technology platform that relies on vaporous atoms, interrogated with laser beams and nearly ionized, to receive rf signals. Rydberg rf sensors have a number of interesting fundamental distinctions from traditional receiver technologies, such as those based on metallic antennas, since they are governed by the quantum physics of atom-light interactions. As Rydberg sensors quickly advance from laboratory experiments into fieldable devices, there is a need for a general software modeling tool that fully encompasses the internal physics of the sensor. The Rydberg Interactive Quantum Module (RydIQule) is a Python package designed to fill this need. The initial public release of RydIQule in late 2023 built the core functionality described above. Here we outline RydIQule's version 2 release which expands on its capabilities to more accurately model real-world atoms.